论文标题

INSE中依赖层的光学诱导的自旋极化

Layer-dependent optically-induced spin polarization in InSe

论文作者

Nelson, Jovan, Stanev, Teodor K., Lebedev, Dmitry, LaMountain, Trevor, Gish, J. Tyler, Zeng, Hongfei, Shin, Hyeondeok, Heinonen, Olle, Watanabe, Kenji, Taniguchi, Takashi, Hersam, Mark C., Stern, Nathaniel P.

论文摘要

使用III-V和II-VI半导体的纳米结构进行了对半导体中自旋的光学控制,但是二维范德华材料的出现为自旋现象提供了另一种低维平台。硫化剂(INSE)是III组单钙化剂范德华材料,由于其高电子迁移率,可调的直接带隙和量子运输,因此对光电的材料显示了有望。有关于自旋依赖性的光学选择规则的预测,这表明在二维分层材料中对自旋的全光激发和控制的潜力。尽管有这些预测,但INSE中的层依赖性光自旋现象尚未探索。在这里,我们介绍了几层和散装INSE中层依赖性光学自旋动力学的测量。偏振光发光揭示了自旋的层依赖性光学取向,从而在几层INSE中证明了光学选择规则。还使用时间分辨的Kerr旋转光谱学在多层INSE中研究了自旋动力学。通过将平面外和平面静态磁场应用于极化的发射测量和KERR测量,提取了INSE的$ G $ -FACTOR。进一步的研究是通过使用$ \ textbf {k} \ cdot \ textbf {p} $模型来计算进动值来完成的,该模型由\ textit {ab-initio}密度函数理论支持。对预测率与实验测量结果的比较突出了激子效应在INSE中对理解自旋动态的重要性。自旋的光学取向是光旋转现象和设备的重要先决条件,并且这些对层依赖性的光学激发的首次证明是将层依赖性依赖性自旋特性与该材料中发现的有利的电子特性相结合的基础。

Optical control of spin in semiconductors has been pioneered using nanostructures of III-V and II-VI semiconductors, but the emergence of two-dimensional van der Waals materials offers an alternative low-dimensional platform for spintronic phenomena. Indium selenide (InSe), a group-III monochalcogenide van der Waals material, has shown promise for opto-electronics due to its high electron mobility, tunable direct bandgap, and quantum transport. There are predictions of spin-dependent optical selection rules suggesting potential for all-optical excitation and control of spin in a two-dimensional layered material. Despite these predictions, layer-dependent optical spin phenomena in InSe have yet to be explored. Here, we present measurements of layer-dependent optical spin dynamics in few-layer and bulk InSe. Polarized photoluminescence reveals layer-dependent optical orientation of spin, thereby demonstrating the optical selection rules in few-layer InSe. Spin dynamics are also studied in many-layer InSe using time-resolved Kerr rotation spectroscopy. By applying out-of-plane and in-plane static magnetic fields for polarized emission measurements and Kerr measurements, respectively, the $g$-factor for InSe was extracted. Further investigations are done by calculating precession values using a $\textbf{k} \cdot \textbf{p}$ model, which is supported by \textit{ab-initio} density functional theory. Comparison of predicted precession rates with experimental measurements highlights the importance of excitonic effects in InSe for understanding spin dynamics. Optical orientation of spin is an important prerequisite for opto-spintronic phenomena and devices, and these first demonstrations of layer-dependent optical excitation of spins in InSe lay the foundation for combining layer-dependent spin properties with advantageous electronic properties found in this material.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源