论文标题

最终用于接触单个原子石墨烯纳米纤维的电极

Ultimately-scaled electrodes for contacting individual atomically-precise graphene nanoribbons

论文作者

Zhang, Jian, Qian, Liu, Barin, Gabriela Borin, Daaoub, Abdalghani H. S., Chen, Peipei, Müllen, Klaus, Sangtarash, Sara, Ruffieux, Pascal, Fasel, Roman, Sadeghi, Hatef, Zhang, Jin, Calame, Michel, Perrin, Mickael L.

论文摘要

自下而上的合成石墨烯纳米纤维(GNR)是量子材料,可以用原子精度进行结构,从而提供了对其物理特性的前所未有的控制。访问GNR的固有功能进行量子技术应用需要在单个GNR级别操纵单电荷,旋转或光子。但是,在实验上,由于其纳米尺寸的宽度和长度以及金属生长底物的高密度,接触单个GNR仍然具有挑战性。在这里,我们证明了使用单壁碳纳米管(SWNT)作为最终缩放的电极在多门设备体系结构中单个GNR的接触和电气表征。 GNR-SWNT设备表现出明确定义的量子传输现象,包括库仑阻断,激发状态和弗兰克 - 康登封锁,所有特征都指向单个GNR的接触。结合多门结构,这种接触方法为量子设备中GNR的整合开辟了道路,以利用其拓扑琐碎和非琐碎的性质。

Bottom-up synthesized graphene nanoribbons (GNRs) are quantum materials that can be structured with atomic precision, providing unprecedented control over their physical properties. Accessing the intrinsic functionality of GNRs for quantum technology applications requires the manipulation of single charges, spins, or photons at the level of an individual GNR. However, experimentally, contacting individual GNRs remains challenging due to their nanometer-sized width and length as well as their high density on the metallic growth substrate. Here, we demonstrate the contacting and electrical characterization of individual GNRs in a multi-gate device architecture using single-walled carbon nanotubes (SWNTs) as ultimately-scaled electrodes. The GNR-SWNT devices exhibit well-defined quantum transport phenomena, including Coulomb blockade, excited states, and Franck-Condon blockade, all characteristics pointing towards the contacting of an individual GNR. Combined with the multi-gate architecture, this contacting method opens a road for the integration of GNRs in quantum devices to exploit their topologically trivial and non-trivial nature.

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