论文标题
局部评论:从实验数据中提取分子框架光电离
Topical Review: Extracting Molecular Frame Photoionization Dynamics from Experimental Data
论文作者
论文摘要
概述和讨论了分子框架(MF)光电离动力学的实验重建方法(MF)光电离心动力学以及相关特性 - 特别是MF光电子角分布(PAD)和连续密度矩阵的方法。引入了非专家阅读器的一般概念,实验和理论技术在某种程度上进一步概述。特定的重点放在用于从时间域元素检索的数值重建技术的详细示例上代码(\ textIt {Photelectron Metrology Toolkit},用Python编写,与PotheLectRons/potherectrons/cosity Splance/EcoSystem一起使用\ textit {量子{量子{Quantit {QuantiT {量子计量学),并通过在线存储库来进行文献;
Methods for experimental reconstruction of molecular frame (MF) photoionization dynamics, and related properties - specifically MF photoelectron angular distributions (PADs) and continuum density matrices - are outlined and discussed. General concepts are introduced for the non-expert reader, and experimental and theoretical techniques are further outlined in some depth. Particular focus is placed on a detailed example of numerical reconstruction techniques for matrix-element retrieval from time-domain experimental measurements making use of rotational-wavepackets (i.e. aligned frame measurements) - the ``bootstrapping to the MF" methodology - and a matrix-inversion technique for direct MF-PAD recovery. Ongoing resources for interested researchers are also introduced, including sample data, reconstruction codes (the \textit{Photoelectron Metrology Toolkit}, written in python, and associated \textit{Quantum Metrology with Photoelectrons} platform/ecosystem), and literature via online repositories; it is hoped these resources will be of ongoing use to the community.