论文标题

在整体上的范德华的连续体中,与自杂交结合状态的强烈互动

Strong light-matter interaction with self-hybridized bound states in the continuum in monolithic van der Waals metasurfaces

论文作者

Weber, Thomas, Kühner, Lucca, Sortino, Luca, Mhenni, Amine Ben, Wilson, Nathan P., Kühne, Julius, Finley, Jonathan J., Maier, Stefan A., Tittl, Andreas

论文摘要

连续体(BICS)中的光子绑定状态是与过渡金属二甲化元素(TMDC)相结合的杰出纳米光子平台,但到目前为止,主要用作全型递质元素,与邻近的TMDC层,与TMDC层相邻的TMDC层,与应变,模式,模式重叠和物质集成相关。在这项工作中,我们在实验上首次证明了不对称依赖性的BIC共振在2D阵列的单片跨面阵列中,仅由纳米结构化的大量TMDC WS $ _2 $与BIC模式呈现出锋利和剪裁的线路,理想增强轻度互动的理想。几何变化可以以散装WS $ _2 $中激子共振的BIC共振进行调整,从而揭示了具有反划入模式的强耦合方案和116 MEV的Rabi分裂。利用BIC概念对BIC概念提供的辐射损失通道的精确控制,可以通过元图的几何不对称参数来量身定制RABI分裂。至关重要的是,耦合强度本身可以受到控制,并且被证明与材料内部损失无关。我们的BIC驱动整体式跨表面平台可以很容易地合并其他TMDC或激子材料,以提供以前不可用的基本见解和用于极化应用程序的实用设备概念。

Photonic bound states in the continuum (BICs) are a standout nanophotonic platform for strong light-matter coupling with transition metal dichalcogenides (TMDCs), but have so far mostly been employed as all-dielectric metasurfaces with adjacent TMDC layers, incurring limitations related to strain, mode overlap, and material integration. In this work, we experimentally demonstrate for the first time asymmetry-dependent BIC resonances in 2D arrays of monolithic metasurfaces composed solely of the nanostructured bulk TMDC WS$_2$ with BIC modes exhibiting sharp and tailored linewidths, ideal for selectively enhancing light-matter interactions. Geometrical variation enables the tuning of the BIC resonances across the exciton resonance in bulk WS$_2$, revealing the strong-coupling regime with an anti-crossing pattern and a Rabi splitting of 116 meV. The precise control over the radiative loss channel provided by the BIC concept is harnessed to tailor the Rabi splitting via a geometrical asymmetry parameter of the metasurface. Crucially, the coupling strength itself can be controlled and is shown to be independent of material-intrinsic losses. Our BIC-driven monolithic metasurface platform can readily incorporate other TMDCs or excitonic materials to deliver previously unavailable fundamental insights and practical device concepts for polaritonic applications.

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