论文标题
快速多重超快非线性显微镜用于材料表征
Rapid multiplex ultrafast nonlinear microscopy for material characterization
论文作者
论文摘要
我们通过测量其非线性响应,激子dephasing和激子寿命来评估高级材料的质量,以根据四波混合(FWM)进行快速成像。我们使用由化学蒸气沉积生长的WSE $ _2 $单层作为证明这些功能的规范示例。相比之下,我们表明,提取材料参数,例如FWM强度,消化时间,激发的状态寿命以及黑暗/局部状态的分布,可以比当前普遍的技术更准确地评估样品质量,包括白光显微镜和线性微反射光谱谱。我们通过建模指数衰减的鲁棒性适合于采样点的不同间距,进一步讨论超快FWM技术的未来改进。实时在室温下实时采用超快非线性成像具有快速现场样品表征的高级材料及其他方式的潜力。
We demonstrate rapid imaging based on four-wave mixing (FWM) by assessing the quality of advanced materials through measurement of their nonlinear response, exciton dephasing, and exciton lifetimes. We use a WSe$_2$ monolayer grown by chemical vapor deposition as a canonical example to demonstrate these capabilities. By comparison, we show that extracting material parameters such as FWM intensity, dephasing times, excited state lifetimes, and distribution of dark/localized states allows for a more accurate assessment of the quality of a sample than current prevalent techniques, including white light microscopy and linear micro-reflectance spectroscopy. We further discuss future improvements of the ultrafast FWM techniques by modeling the robustness of exponential decay fits to different spacing of the sampling points. Employing ultrafast nonlinear imaging in real-time at room temperature bears the potential for rapid in-situ sample characterization of advanced materials and beyond.