论文标题

S = 1/2的QUASIKAGOME晶格CERH1-XPDXSN中的量子临界旋转液样行为,使用MUON自旋松弛和中子散射研究

Quantum critical spin-liquid-like behavior in S = 1/2 quasikagome lattice CeRh1-xPdxSn investigated using muon spin relaxation and neutron scattering

论文作者

Tripathi, Rajesh, Adroja, D. T., Ritter, C., Sharma, Shivani, Yang, Chongli, Hillier, A. D., Koza, M. M., Demmel, F., Sundaresan, A., Langridge, S., Higemoto, Wataru, Ito, Takashi U., Strydom, A. M., Stenning, G. B. G., Bhattacharyya, A., Keen, David, Walker, H. C., Perry, R. S., Pratt, Francis, Si, Qimiao, Takabatake, T.

论文摘要

我们介绍了Muon Spin放松($μ$ SR)和基于CE的Quasikagome晶格CERH $ _ {1-x} $ pd $ _ {x} $ sn($ x = 0.1 $ to 0.75)上的MUON SPIN放松($μ$ SR)和中子散射的结果。我们的ZF- $μ$ SR结果显示,静态远程磁性顺序的缺乏降至0.05〜K,$ x = 0.1 $单晶。动态自旋波动的弱温度依赖性平台低于0.2〜 k,ZF- $μ$ SR及其纵向场(LF)依赖性在0和3〜 kg之间的依赖性,即使在$ = 0.05〜k的情况下,动态自旋波动也持续存在,即使没有静态磁性顺序。另一方面,$ c _ {\ text {4f}} $/$ t $在0.9〜k以下冷却时以-log $ t $的增加,在0.13〜K下通过广泛的最大值,并在进一步冷却时略微降低。 AC敏感性还表现出0.16〜K处的频率独立宽峰值,这在$ C $方向上是在应用的场上$ h $的突出峰。因此,我们认为,$ x = 0.1 $的这种行为(即,旋转放松率($λ$)低于0.2〜k的高原($λ$)和$ c _ {\ text {4f}} $ 0.13〜k以下的线性$ t $依赖性可以归因于金属旋转式(sl)的基础,这是一个沮丧的点状态。 LF- $ $ $ SR的研究表明,kagome平面旋转波动是造成SL行为的原因。 $ x $ = 0.1的低能量非弹性中子散射(INS)揭示了无间隙的磁激发,这也由$ c _ {\ text {4f}} $与$ t^{1.1} $成比例的行为所支持。

We present the results of muon spin relaxation ($μ$SR) and neutron scattering on the Ce-based quasikagome lattice CeRh$_{1-x}$Pd$_{x}$Sn ($x=0.1$ to 0.75). Our ZF-$μ$SR results reveal the absence of static long-range magnetic order down to 0.05~K in $x = 0.1$ single crystals. The weak temperature-dependent plateaus of the dynamic spin fluctuations below 0.2~K in ZF-$μ$SR together with its longitudinal-field (LF) dependence between 0 and 3~kG indicate the presence of dynamic spin fluctuations persisting even at $T$ = 0.05~K without static magnetic order. On the other hand, $C_{\text{4f}}$/$T$ increases as --log $T$ on cooling below 0.9~K, passes through a broad maximum at 0.13~K and slightly decreases on further cooling. The ac-susceptibility also exhibits a frequency independent broad peak at 0.16~K, which is prominent with an applied field $H$ along $c$-direction. We, therefore, argue that such a behavior for $x=0.1$ (namely, a plateau in spin relaxation rate ($λ$) below 0.2~K and a linear $T$ dependence in $C_{\text{4f}}$ below 0.13~K) can be attributed to a metallic spin-liquid (SL) ground state near the quantum critical point in the frustrated Kondo lattice. The LF-$μ$SR study suggests that the out of kagome plane spin fluctuations are responsible for the SL behavior. Low energy inelastic neutron scattering (INS) of $x$ = 0.1 reveals gapless magnetic excitations, which are also supported by the behavior of $C_{\text{4f}}$ proportional to $T^{1.1}$ down to 0.06~K.

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