论文标题

单晶2D材料纳米替宾网络用于纳米电子学

Single Crystalline 2D Material Nanoribbon Networks for Nanoelectronics

论文作者

Aslam, Muhammad Awais, Tran, Tuan Hoang, Supina, Antonio, Siri, Olivier, Meunier, Vincent, Watanabe, Kenji, Taniguchi, Takashi, Kralj, Marko, Teichert, Christian, Sheremet, Evgeniya, Rodriguez, Raul D., Matković, Aleksandar

论文摘要

在过去的十年中,由于它们在量子领域中的潜在应用,与石墨烯纳米容器有关的一系列研究。然而,由于没有合成途径,几乎没有报道其他2D材料的纳米容器的实验性工作。在这里,我们提出了一种普遍的方法,可以从任意2D材料中合成纳米管的高质量网络,同时保持高结晶度,足够的产量,狭窄的尺寸分布和直接前向设备的集成性。通过制造MOS2,WS2,WSE2和石墨烯纳米替伯侧效应晶体管,这些技术的广泛适用性可以证明,这些晶体固有地不会遭受互连电阻。通过依靠自组装和自我对准的有机纳米结构作为掩盖,我们证明了控制纳米替比边缘的主要晶体学方向的可能性。电气表征显示出创纪录的迁移率,尽管宽度极高,但对于各种TMDC的电流都非常高。最后,我们探索具有纳米替比边缘的装饰,该纳米纤维边缘具有等离子颗粒,为开发纳米吡啶的等离激元传感和光电设备的装饰。

The last decade has seen a flurry of studies related to graphene nanoribbons owing to their potential applications in the quantum realm. However, little experimental work has been reported towards nanoribbons of other 2D materials due to the absence of synthesis routes. Here, we propose a universal approach to synthesize high-quality networks of nanoribbons from arbitrary 2D materials while maintaining high crystallinity, sufficient yield, narrow size distribution, and straight-forward device integrability. The wide applicability of this technique is demonstrated by fabricating MoS2, WS2, WSe2, and graphene nanoribbon field effect transistors that inherently do not suffer from interconnection resistances. By relying on self-assembled and self-aligned organic nanostructures as masks, we demonstrate the possibility of controlling the predominant crystallographic direction of the nanoribbon's edges. Electrical characterization shows record mobilities and very high ON currents for various TMDCs despite extreme width scaling. Lastly, we explore decoration of nanoribbon edges with plasmonic particles paving the way towards the development of nanoribbon-based plasmonic sensing and opto-electronic devices.

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