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The notion of non-deterministic logical matrix (where connectives are interpreted as multi-functions) preserves many good properties of traditional semantics based on logical matrices (where connectives are interpreted as functions) whilst finitely characterizing a much wider class of logics, and has proven to be decisive in a myriad of recent compositional results in logic. Crucially, when a finite non-deterministic matrix satisfies monadicity (distinct truth-values can be separated by unary formulas) one can automatically produce an axiomatization of the induced logic. Furthermore, the resulting calculi are analytical and enable algorithmic proof-search and symbolic counter-model generation. For finite (deterministic) matrices it is well known that checking monadicity is decidable. We show that, in the presence of non-determinism, the property becomes undecidable. As a consequence, we conclude that there is no algorithm for computing the set of all multi-functions expressible in a given finite Nmatrix. The undecidability result is obtained by reduction from the halting problem for deterministic counter machines.