论文标题

石墨烯 - 单层XENON异质结构中的原位可调节高阶模式来量身定制狄拉克费米。

Tailoring Dirac fermions by in-situ tunable high-order moire pattern in graphene-monolayer xenon heterostructure

论文作者

Wu, Chunlong, Wan, Qiang, Peng, Cao, Mo, Shangkun, Li, Renzhe, Zhao, Keming, Guo, Yanping, Yuan, Shengjun, Wu, Fengcheng, Zhang, Chendong, Xu, Nan

论文摘要

最近,在扭曲双层石墨烯(TBLG)和其他Moire超级晶格中,已经实现了各种新型量子相,包括相关的绝缘子,超导性,磁性和拓扑状态。这些现象对Moire超级晶格非常敏感,几乎无法快速或强烈地更改。在这里,我们报告了石墨烯 - 单层XENON异质结构(G/MXE)中高阶Moire模式(高阶干扰模式)的实验实现,Moire周期通过不同的退火温度和压力来改变XE的lattice常数,从几个纳米到无限的含量。我们使用角度分辨的光发射光谱直接观察到石墨烯狄拉克锥的复制品出现并在动量空间中彼此靠近,因为Moire模式在真实空间中不断扩展。当Moire时期接近无穷大时,副本最终彼此重叠,并且在Intertley耦合引起的狄拉克点上观察到一个能隙,这是Kekule失真的表现。我们构建了连续的莫伊尔汉密尔顿人,可以很好地解释实验结果。 G/MXE中Moire Hamiltonian的形式与TBLG中的形式相似,并且在G/MXE中预测具有狭窄带宽的Moire带。但是,来自G/MXE的不同山谷的Moire Hamiltonian夫妇Dirac Fermions,而不是来自TBLG的不同层的Fermions。我们的工作展示了一个新的平台,可以研究Moire模式的连续演变及其对电子结构的调制效果,并提供了一种前所未有的方法,可通过可调间隔耦合来调整Dirac Fermions。

A variety of novel quantum phases have been achieved in twist bilayer graphene (tBLG) and other moire superlattices recently, including correlated insulators, superconductivity, magnetism, and topological states. These phenomena are very sensitive to the moire superlattices, which can hardly be changed rapidly or intensely. Here, we report the experimental realization of a high-order moire pattern (a high-order interference pattern) in graphene-monolayer xenon heterostructure (G/mXe), with moire period in-situ tuned from few nanometers to infinity by changing the lattice constant of Xe through different annealing temperatures and pressures. We use angle-resolved photoemission spectroscopy to directly observe that replicas of graphene Dirac cone emerge and move close to each other in momentum-space as moire pattern continuously expands in real-space. When the moire period approaches infinity, the replicas finally overlap with each other and an energy gap is observed at the Dirac point induced by intervalley coupling, which is a manifestation of Kekule distortion. We construct a continuum moire Hamiltonian, which can explain the experimental results well. The form of moire Hamiltonian in G/mXe is similar to that in tBLG, and moire band with narrow bandwidth is predicted in G/mXe. However, the moire Hamiltonian couples Dirac fermions from different valleys in G/mXe, instead of ones from different layers in tBLG. Our work demonstrates a novel platform to study the continuous evolution of moire pattern and its modulation effect on electronic structure, and provides an unprecedented approach for tailoring Dirac fermions with tunable intervalley coupling.

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