论文标题

使用甲基橙色有机染料溶液的快速和热中子的相互作用过程的研究

Research of interaction processes of fast and thermal neutrons with solution of methyl orange organic dye

论文作者

Gokov, Sergey P., Kazarinov, Yuri G., Kalenik, Sergiy A., Kasilov, Valentin Y., Malykhina, Tetiana V., Rudychev, Yegor V., Tsiatsko, Vitaliy V.

论文摘要

已经研究了与甲基橙色有机染料水溶液相互作用的中子通量的过程。这项工作是在NSC KIPT的Linac Lue-300上进行的。一组钨板用作中子生成目标。电子能量为15 meV,平均电流为20 mka。样品位于铅盾牌后面,没有主持人,没有它。使用GEANT4工具包进行此实验,中子通量及其能量光谱是在没有主持人和不同厚度(1-5 cm)的主持人的实验样品的位置计算的。对实验结果的分析表明,当没有铅屏蔽和没有主持人的物体被照射时,染料分子就会完全破坏。在存在铅保护的情况下,观察到染料分子的10%破坏。当铅屏蔽后面安装了五厘米聚乙烯主持人时,实际上未观察到没有硼酸在热中子上的染料分子的破坏。当热和表皮中子的通量与含有4%硼酸的染料溶液相互作用时,由于放热反应10b(n,a),观察到染料分子的30%破坏。该研究表明,有机染料的溶液是创建用于记录热中性和表皮中子通量的探测器的良好材料。此类探测器可用于对环境,核动力工程和核医学以及中子捕获治疗研究领域的环境监测。

The processes of neutron fluxes interaction with an aqueous solution of methyl orange organic dye have been investigated. The work was carried out on a LINAC LUE-300 at NSC KIPT. A set of tungsten plates was used as a neutron-generating target. The electron energy was 15 MeV, the average current was 20 mkA. The samples were located behind the lead shield and without it, with and without a moderator. Using the Geant4 toolkit for this experiment, neutron fluxes and their energy spectra were calculated at the location of experimental samples without a moderator and with a moderator of different thickness (1-5 cm). An analysis of the experimental results showed that when objects without lead shielding and without a moderator are irradiated, the dye molecules are completely destroyed. In the presence of lead protection, 10% destruction of the dye molecules was observed. When a five-centimeter polyethylene moderator was installed behind the lead shield, the destruction of dye molecules without boric acid on thermal neutrons was practically not observed. When the fluxes of thermal and epithermal neutrons interacted with a dye solution containing 4% boric acid, 30% destruction of dye molecules was observed due to the exothermic reaction 10B (n, a). The research has shown that solutions of organic dyes are a good material for creating detectors for recording fluxes of thermal and epithermal neutrons. Such detectors can be used for radioecological monitoring of the environment, in nuclear power engineering and nuclear medicine, and in the field of neutron capture therapy research in particular.

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