论文标题
光子量子技术的单个有机分子
Single organic molecules for photonic quantum technologies
论文作者
论文摘要
在固态中分离单分子已允许在基础科学和应用科学中进行基本实验。当冷却至液态氦温度时,某些分子显示过过渡线,这些过渡线是数十兆赫兹宽的过渡线,仅受激发态寿命的限制。有机材料合成的极端灵活性以低成本提供了宽阔的发射波长和支持矩阵的宽面条。在过去的几十年中,与光子结构的受控耦合导致了与光的优化相互作用效率。因此,分子可以作为单个光子源和具有竞争性能的非线性元素操作,该元素在相干性,可伸缩性和与各种集成平台的兼容性方面都可以运行。此外,它们可以用作磁场和材料特性的光学读数的换能器,并有望在传感和运动的传感中分辨率分辨率。我们表明,基于单分子的量子发射器有望在量子科学和技术的发展中发挥关键作用。
Isolating single molecules in the solid state has allowed fundamental experiments in basic and applied sciences. When cooled down to liquid helium temperature, certain molecules show transition lines, that are tens of megahertz wide, limited only by the excited state lifetime. The extreme flexibility in the synthesis of organic materials provides, at low costs, a wide palette of emission wavelengths and supporting matrices for such single chromophores. In the last decades, the controlled coupling to photonic structures has led to an optimized interaction efficiency with light. Molecules can hence be operated as single photon sources and as non-linear elements with competitive performance in terms of coherence, scalability and compatibility with diverse integrated platforms. Moreover, they can be used as transducers for the optical read-out of fields and material properties, with the promise of single-quanta resolution in the sensing of charges and motion. We show that quantum emitters based on single molecules hold promise to play a key role in the development of quantum science and technologies.