论文标题

在沮丧的自旋1/2链中的热效应与自旋源性

Thermal effects versus spin nematicity in a frustrated spin-1/2 chain

论文作者

Pregelj, M., Zorko, A., Arčon, D., Klanjšek, M., Zaharko, O., Krämer, S., Horvatić, M., Prokofiev, A.

论文摘要

旋转阶段是一种有趣的物质状态,缺乏通常的远程偶极阶,但它显示出较高的多极顺序。这使得其检测极为困难和有争议。最近,已提出核磁共振(NMR)是确认其存在的最合适的技术之一。我们报告了$^{17} $ o nmr观察在沮丧的Spin-1/2链的两极分化状态下还原局部磁化的$β$β$ -TEVO $ _4 $,以前被认为是旋转纽扣行为的指纹。然而,我们的详细研究表明,通过NMR频移探测的磁化的缺失部分被热激活,从而破坏了所研究化合物中自旋纽的存在。这凸显了仔细考虑温度依赖性的NMR转移的重要性,而NMR转移在先前的自旋列性研究中已经忽略了。

The spin-nematic phase is an intriguing state of matter that lacks usual long-range dipolar order, yet it exhibits higher multipolar order. This makes its detection extremely difficult and controversial. Recently, nuclear magnetic resonance (NMR) has been proposed as one of the most suitable techniques to confirm its existence. We report a $^{17}$O NMR observation of the reduction of the local magnetization in the polarized state of the frustrated spin-1/2 chain $β$-TeVO$_4$, which was previously proposed to be a fingerprint of the spin-nematic behavior. However, our detailed study shows that the detected missing fraction of the magnetization, probed by NMR frequency shift, is thermally activated, thus undermining the presence of the spin-nematic phase in the investigated compound. This highlights the importance of careful considerations of temperature-dependent NMR shift that has been overlooked in previous studies of spin nematicity.

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