论文标题

超快粘度测量与弹道光镊

Ultrafast viscosity measurement with ballistic optical tweezers

论文作者

Madsen, Lars S., Waleed, Muhammad, Casacio, Catxere A., Stilgoe, Alexander B., Taylor, Michael A., Bowen, Warwick P.

论文摘要

粘度是非平衡系统的重要特性,例如活性生物材料和驱动的非牛顿流体,以及从生物材料到地质,能源技术和医学的田地。但是,非侵入性粘度测量通常需要秒的整合时间。在这里,我们证明了速度的四个速度提高,低至二十微秒,不确定性首次由基本热噪声支配。我们使用光学镊子中被困粒子的瞬时速度实现了这一目标。为了解决瞬时速度,我们开发了一个结构化的检测系统,该系统允许使用Megahertz带宽进行粒子跟踪。我们的结果将粘度从静态平均属性转化为可能在活动动力学的时间标准上动态跟踪的粘度。这为从平衡系统(从相变的快速动力学到运动分子步进中的能量耗散)到违反平衡热力学的波动法则的途径打开了新发现的途径。

Viscosity is an important property of out-of-equilibrium systems such as active biological materials and driven non-Newtonian fluids, and for fields ranging from biomaterials to geology, energy technologies and medicine. However, noninvasive viscosity measurements typically require integration times of seconds. Here we demonstrate a four orders-of-magnitude improvement in speed, down to twenty microseconds, with uncertainty dominated by fundamental thermal noise for the first time. We achieve this using the instantaneous velocity of a trapped particle in an optical tweezer. To resolve the instantaneous velocity we develop a structured-light detection system that allows particle tracking with megahertz bandwidths. Our results translate viscosity from a static averaged property, to one that may be dynamically tracked on the timescales of active dynamics. This opens a pathway to new discoveries in out-of-equilibrium systems, from the fast dynamics of phase transitions, to energy dissipation in motor molecule stepping, to violations of fluctuation laws of equilibrium thermodynamics.

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