论文标题

液滴中的涡流驱动动力学

The vortex-driven dynamics of droplets within droplets

论文作者

Tiribocchi, A., Montessori, A., Lauricella, M., Bonaccorso, F., Succi, S., Aime, S., Milani, M., Weitz, D. A.

论文摘要

了解流体结构相互作用对于软中尺度材料的最佳设计和制造至关重要。多核乳液是一类软体流体,这些液体是由可变形的油水双液滴(核心)组装而成的,通常用作建筑块,用于实现生物技术感兴趣的设备,例如药物 - 释放,组织工程和再生药物。在这里,我们研究了微流体通道中流动的多核乳液的物理学,并报告了多种驱动的非平衡状态(NES)的数值证据,其形成是由偶性流体涡流引起的,该偶性流体是由微电脑内流动载体剪切结构触发的。观察到的动态状态范围从低核心区域分数的长寿命NES,其为特征,其特征是内部滴的行星样运动,到高核区域级分的短寿命,其中与自我稳态的流体动力相互作用结合了内部滴度的多体体碰撞。骨质前行为的发作以从一个涡流到另一个涡流的核心过渡标志着,我们将其解释为系统的表现,以通过填充胶囊在胶囊中动态出现的空隙来最大化其熵。

Understanding the fluid-structure interaction is crucial for an optimal design and manufacturing of soft mesoscale materials. Multi-core emulsions are a class of soft fluids assembled from cluster configurations of deformable oil-water double droplets (cores), often employed as building-blocks for the realisation of devices of interest in bio-technology, such as drug-delivery, tissue engineering and regenerative medicine. Here, we study the physics of multi-core emulsions flowing in microfluidic channels and report numerical evidence of a surprisingly rich variety of driven non-equilibrium states (NES), whose formation is caused by a dipolar fluid vortex triggered by the sheared structure of the flow carrier within the microchannel. The observed dynamic regimes range from long-lived NES at low core-area fraction, characterised by a planetary-like motion of the internal drops, to short-lived ones at high core-area fraction, in which a pre-chaotic motion results from multi-body collisions of inner drops, as combined with self-consistent hydrodynamic interactions. The onset of pre-chaotic behavior is marked by transitions of the cores from one vortex to another, a process that we interpret as manifestations of the system to maximize its entropy by filling voids, as they arise dynamically within the capsule.

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