论文标题

时钟螺旋钻电子

Clocking Auger Electrons

论文作者

Haynes, D. C., Wurzer, M., Schletter, A., Al-Haddad, A., Blaga, C., Bostedt, C., Bozek, J., Bucher, M., Camper, A., Carron, S., Coffee, R., Costello, J. T., DiMauro, L. F., Ding, Y., Ferguson, K., Grguraš, I., Helml, W., Hoffmann, M. C., Ilchen, M., Jalas, S., Kabachnik, N. M., Kazansky, A. K., Kienberger, R., Maier, A. R., Maxwell, T., Mazza, T., Meyer, M., Park, H., Robinson, J. S., Roedig, C., Schlarb, H., Singla, R., Tellkamp, F., Zhang, K., Doumy, G., Behrens, C., Cavalieri, A. L.

论文摘要

激烈的X射线自由电子激光器(XFELS)可以迅速激发物质,使其处于固有的不稳定状态,这些状态在飞秒时尺度上衰减。由于放松主要通过螺旋钻的发射发生,因此激发状态观测值受螺旋腐烂的限制。因此,该过程的原位测量至关重要,但是由于固有的时机和相位抖动,在Xfels上仍然难以捉摸,这可能是比螺旋杆衰减的时间尺度大的数量级。在这里,我们基于对条纹的照片和螺旋钻电子的同时测量,开发了一种新的方法,称为自我引用的attosent条纹。尽管有抖动,我们的技术仍可以次秒。我们利用这种方法来制作原子霓虹灯中螺旋蛋白衰变寿命的第一个XFEL时间域测量,并通过使用完全量子力学描述,检索Kll Decay decay通道的寿命为$ 2.2^{ + 0.2} _ { - 0.3} $ fs。重要的是,我们的技术可以推广,以允许将AttSeent时间分辨的实验扩展到所有当前和将来的FEL设施。

Intense X-ray free-electron lasers (XFELs) can rapidly excite matter, leaving it in inherently unstable states that decay on femtosecond timescales. As the relaxation occurs primarily via Auger emission, excited state observations are constrained by Auger decay. In situ measurement of this process is therefore crucial, yet it has thus far remained elusive at XFELs due to inherent timing and phase jitter, which can be orders of magnitude larger than the timescale of Auger decay. Here, we develop a new approach termed self-referenced attosecond streaking, based upon simultaneous measurements of streaked photo- and Auger electrons. Our technique enables sub-femtosecond resolution in spite of jitter. We exploit this method to make the first XFEL time-domain measurement of the Auger decay lifetime in atomic neon, and, by using a fully quantum-mechanical description, retrieve a lifetime of $2.2^{ + 0.2}_{ - 0.3}$ fs for the KLL decay channel. Importantly, our technique can be generalised to permit the extension of attosecond time-resolved experiments to all current and future FEL facilities.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源