论文标题
二维磁绝缘子异源异常响应量量异常效应
Quantum anomalous Hall effect in two-dimensional magnetic insulator heterojunctions
论文作者
论文摘要
近年来,在发现物质的拓扑状态中取得了巨大的成功。特别是,已经开发了时间反向不变拓扑阶段的复杂理论方法,从而全面搜索了水晶数据库和数千种新的拓扑材料的预测。相比之下,由于磁性和拓扑电子带的共存,在单个化合物中很少发现磁性逆转的磁性拓扑阶段,因为磁性逆转仍然局限于几种模范材料。为了克服这一挑战,我们提出了一种替代方法来实现量子异常效果(QAH)效应,这是磁性拓扑阶段的一个典型示例,通过工程二维(2D)磁性van der wa waals杂点。而不是单个磁性拓扑材料,我们搜索具有特定带对齐方式的两个2D(通常是微不足道的)磁性绝缘子化合物的组合,以便它们可以与拓扑非琐事的带状结构一起形成类型的III II II异质结。 By combining the data-driven materials search, first principles calculations, and the symmetry-based analytical models, we identify 8 type-III heterojunctions consisting of 2D ferromagnetic insulator materials from a family of 2D monolayer MXY compounds (M = metal atoms, X = S, Se, Te, Y = F, Cl, Br, I) as a set of candidates for the QAH effect.特别是,我们直接计算MNNF/MNNCL异质结中的拓扑不变(Chern数)和手性边缘状态,并具有铁磁堆叠。这项工作说明了如何将数据驱动的材料科学与基于对称性的物理原理结合在一起,以指导搜索新型基于异质结的量子材料,该量子托有QAH效应和其他外来量子状态。
Recent years have witnessed tremendous success in the discovery of topological states of matter. Particularly, sophisticated theoretical methods in time-reversal-invariant topological phases have been developed, leading to the comprehensive search of crystal database and the prediction of thousands of new topological materials. In contrast, the discovery of magnetic topological phases that break time reversal is still limited to several exemplary materials because the coexistence of magnetism and topological electronic band structure is rare in a single compound. To overcome this challenge, we propose an alternative approach to realize the quantum anomalous Hall (QAH) effect, a typical example of magnetic topological phase, via engineering two-dimensional (2D) magnetic van der Waals heterojunctions. Instead of a single magnetic topological material, we search for the combinations of two 2D (typically trivial) magnetic insulator compounds with specific band alignment so that they can together form a type-III heterojunction with topologically non-trivial band structure. By combining the data-driven materials search, first principles calculations, and the symmetry-based analytical models, we identify 8 type-III heterojunctions consisting of 2D ferromagnetic insulator materials from a family of 2D monolayer MXY compounds (M = metal atoms, X = S, Se, Te, Y = F, Cl, Br, I) as a set of candidates for the QAH effect. In particular, we directly calculate the topological invariant (Chern number) and chiral edge states in the MnNF/MnNCl heterojunction with ferromagnetic stacking. This work illustrates how data-driven material science can be combined with symmetry-based physical principles to guide the search for novel heterojunction-based quantum materials hosting the QAH effect and other exotic quantum states in general.