论文标题

阶段多样性电磁抽样:单发terahertz波形记录的一种新方法

Phase Diversity Electro-optic Sampling: A new approach to single-shot terahertz waveform recording

论文作者

Roussel, Eléonore, Szwaj, Christophe, Steffen, Bernd, Evain, Clément, Gerth, Christopher, Jalali, Bahram, Bielawski, Serge

论文摘要

THZ光谱法是用于检测食品工业中微生物和有害化合物的新兴工具,生物医学中蛋白质的研究以及用于分子成像和光刻学的电子梁X射线源的发展。在此类应用中不可逆过程的Terahertz光谱以及在频谱的THZ部分中,单发中THZ电场演变的记录至关重要。但是,在长期窗口中实现子秒分辨率是电磁抽样的一个开放问题,这是记录Terahertz波形的标准技术。我们为这个开放问题引入了一个新的概念框架,该框架灵感来自时间拉伸理论。这个新颖的框架揭示了解决这个20岁的问题的解决方案,从而导致了可实现的时间分辨率的巨大增强。我们在两个应用程序中验证了这项新技术。首先,我们介绍了具有创纪录的时间分辨率的长时间自由传播的Terahertz瞬变的单拍录音。其次,我们介绍了欧洲X射线免费电子激光器的超短相对论电子束的录音。这些结果表明,现在可以用Terahertz带宽在任意长的窗口上记录电信号,从而实现了具有任意时间宽宽产品的“单杆Terahertz示波器”和单发时间域光谱系统。

THz spectroscopy is an emerging tool for detection of microorganisms and harmful compounds in the food industry, the study of proteins in biomedicine and the development of electron-beam X-ray sources for molecular imaging and lithography. Recording of THz electric field evolution in single-shot is crucially needed in terahertz spectroscopy of irreversible processes in such applications as well as for data communication in the THz portion of the spectrum where there is an abundance of untapped bandwidth. However, achieving sub-picosecond resolution over a long time window has been an open problem for electro-optic sampling -- the standard technique for recording terahertz waveforms. We introduce a new conceptual framework for this open problem that is inspired by time-stretch theory. The novel framework unveils a solution to this 20 year-old problem leading to a dramatic enhancement of the achievable temporal resolution. We validate this new technology in two applications. First, we present single shot recordings of long free-propagating terahertz transients with record time resolution. Second, we present recordings of ultra-short relativistic electron bunches at the European X-ray Free Electron Laser. These results show that electric signals may be now recorded with terahertz bandwidth over arbitrarily long windows, thus enabling the realization of "single-shot terahertz oscilloscopes" and single-shot time-domain spectroscopy systems with an arbitrary time-bandwidth product.

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